Experimental signature of a topological quantum dot
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Experimental signature of a topological quantum dot. / Rider, Marie S.; Sokolikova, Maria; Hanham, S. M.; Navarro-Cia, Miguel; Haynes, Peter D; Lee, Derek; Daniele, Maddalena; Guidi, Mariangela Cestelli; Mattevi, Cecilia; Lupi, Stefano; Vincenzo, Giannini.
In: Nanoscale, Vol. 12, No. 44, 28.11.2020, p. 22817-22825.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Experimental signature of a topological quantum dot
AU - Rider, Marie S.
AU - Sokolikova, Maria
AU - Hanham, S. M.
AU - Navarro-Cia, Miguel
AU - Haynes, Peter D
AU - Lee, Derek
AU - Daniele, Maddalena
AU - Guidi, Mariangela Cestelli
AU - Mattevi, Cecilia
AU - Lupi, Stefano
AU - Vincenzo, Giannini
PY - 2020/11/28
Y1 - 2020/11/28
N2 - Topological insulator nanoparticles (TINPs) host topologically protected Dirac surface states, just like their bulk counterparts. For TINPs of radius <100 nm, quantum confinement on the surface results in the discretization of the Dirac cone. This system of discrete energy levels is referred to as a topological quantum dot (TQD) with energy level spacing on the order of Terahertz (THz), which is tunable with material-type and particle size. The presence of these discretized energy levels in turn leads to a new electron-mediated phonon-light coupling in the THz range, and the resulting mode can be observed in the absorption cross-section of the TINPs. We present the first experimental evidence of this new quantum phenomenon in Bi2Te3 topological quantum dots, remarkably observed at room temperature.
AB - Topological insulator nanoparticles (TINPs) host topologically protected Dirac surface states, just like their bulk counterparts. For TINPs of radius <100 nm, quantum confinement on the surface results in the discretization of the Dirac cone. This system of discrete energy levels is referred to as a topological quantum dot (TQD) with energy level spacing on the order of Terahertz (THz), which is tunable with material-type and particle size. The presence of these discretized energy levels in turn leads to a new electron-mediated phonon-light coupling in the THz range, and the resulting mode can be observed in the absorption cross-section of the TINPs. We present the first experimental evidence of this new quantum phenomenon in Bi2Te3 topological quantum dots, remarkably observed at room temperature.
KW - topology
KW - terahertz
KW - plasmons
KW - topological insulator
KW - quantum theory
KW - quantum dots
U2 - https://doi.org/10.1039/D0NR06523D
DO - https://doi.org/10.1039/D0NR06523D
M3 - Article
VL - 12
SP - 22817
EP - 22825
JO - Nanoscale
JF - Nanoscale
SN - 2040-3364
IS - 44
ER -