Estimation of particle resuspension source strength on a major London Road

Non-exhaust particles from road traffic arise from both abrasion sources and the resuspension of particles from the road surface. This paper reports a new combination of existing methods for indirect estimation of resuspension emission factors for Marylebone Road, London, a busy multi-lane highway in a street canyon. The method involves firstly estimating the total source strength of coarse particles (PM2.5-10) arising from the road by calculating the roadside incremental concentration of coarse particles above the urban background. This is converted to a source strength by its ratio to NOx whose source strength is estimated from the knowledge of the traffic mix and mean speed. This coarse particle source strength is assumed to represent the sum of resuspension emissions and the coarse particle component of abrasion emissions. Using information on the traffic mix and speed, the abrasion emissions have been calculated from the EMEP/CORINAIR emissions factor database, the result subtracted from the total coarse particle emissions in order to yield resuspension emissions, and combined with traffic count data to derive fleet-average emission factors. Using the fact that the traffic mix differs substantially between weekdays and weekends, separate average emission factors for light- and heavy-duty vehicles have been estimated. In addition to traffic mix, the influence of wind speed and the time elapsed since the last rainfall upon resuspension have been estimated. Wind speed was found to have by far the larger influence, although this was still secondary to the number of heavy-duty vehicles. Uncertainties arising from the choice of urban background site and poor data quality are discussed. (c) 2007 Elsevier Ltd. All rights reserved.