Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs

Nor Arifin; Timothy Button; Robert Steinberger-Wilckens

Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs

Nor Arifin, Timothy Button, Robert Steinberger-Wilckens

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

4 Citations (Scopus)

259 Downloads (Pure)

Abstract

Nickel-Yttria stabilized zirconia (Ni/8YSZ) and Nickel Ceria doped-Scandia stabilised zirconia (Ni/10ScCeSZ) anode supported cells were successfully fabricated using a reverse aqueous tape casting method. The performance of the full cells were tested using both hydrogen and dry biogas at the anode side and ambient air at the cathode side in the temperature range 750°C to 800°C. In hydrogen, Ni/10ScCeSZ showed better performance at 800°C compared to the Ni/8YSZ cell. Switching the fuel from hydrogen to dry biogas, the performance of the Ni/8YSZ cell reduced significantly from 0.31 W/cm2 to 0.06 W/cm2. With Ni/10ScCeSZ cells, the cell performance in biogas was 4 times higher than the corresponding Ni8YSZ cells. The maximum power density decreased only from 0.36 W/cm2 to 0.22 W/cm2 in Ni/10ScCeSZ cell tested when switched from hydrogen to biogas. The results of this work indicate the possibility of using biogas or other carbonaceous fuel in SOFCs without the addition of water (steam).

Original language	English
Title of host publication	Proceedings of SOFC XV
Editors	Subhash C. Singhal, T. Kawada
Place of Publication	Pennington
Publisher	Electrochemical Society Inc.
Pages	1417-1426
Volume	78
Edition	1
ISBN (Electronic)	978-1-62332-457-5
ISBN (Print)	978-1-60768-815-0
Publication status	Published - 23 Jul 2017
Event	15th International Symposium on Solid Oxide Fuel Cells, SOFC, 2017 - Hollywood, FL, U.S.A., Hollywood, United States Duration: 23 Jul 2017 → 28 Jul 2017 http://www.electrochem.org/sofc-xv

Publication series

Name	ECS Transactions
Publisher	ECS
Number	1
Volume	78

Conference

Conference	15th International Symposium on Solid Oxide Fuel Cells, SOFC, 2017
Abbreviated title	SOFC XV
Country/Territory	United States
City	Hollywood
Period	23/07/17 → 28/07/17
Internet address	http://www.electrochem.org/sofc-xv

Keywords

SOFC
tape casting
anode supported SOFC
planar SOFC
aqueous tape casting
Carbon deposition

ASJC Scopus subject areas

Chemical Engineering (miscellaneous)
Materials Chemistry
Fuel Technology

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Anisa SOFC XV FinalAccepted author manuscript, 731 KBLicence: None: All rights reserved

Cite this

@inproceedings{d0603aa6470a48e7b8c9a4664d3aeae0,

title = "Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs",

abstract = "Nickel-Yttria stabilized zirconia (Ni/8YSZ) and Nickel Ceria doped-Scandia stabilised zirconia (Ni/10ScCeSZ) anode supported cells were successfully fabricated using a reverse aqueous tape casting method. The performance of the full cells were tested using both hydrogen and dry biogas at the anode side and ambient air at the cathode side in the temperature range 750°C to 800°C. In hydrogen, Ni/10ScCeSZ showed better performance at 800°C compared to the Ni/8YSZ cell. Switching the fuel from hydrogen to dry biogas, the performance of the Ni/8YSZ cell reduced significantly from 0.31 W/cm2 to 0.06 W/cm2. With Ni/10ScCeSZ cells, the cell performance in biogas was 4 times higher than the corresponding Ni8YSZ cells. The maximum power density decreased only from 0.36 W/cm2 to 0.22 W/cm2 in Ni/10ScCeSZ cell tested when switched from hydrogen to biogas. The results of this work indicate the possibility of using biogas or other carbonaceous fuel in SOFCs without the addition of water (steam).",

keywords = "SOFC, tape casting, anode supported SOFC, planar SOFC, aqueous tape casting, Carbon deposition",

author = "Nor Arifin and Timothy Button and Robert Steinberger-Wilckens",

year = "2017",

month = jul,

day = "23",

language = "English",

isbn = "978-1-60768-815-0",

volume = "78",

series = "ECS Transactions",

publisher = "Electrochemical Society Inc.",

number = "1",

pages = "1417--1426",

editor = "Singhal, {Subhash C.} and T. Kawada",

booktitle = "Proceedings of SOFC XV",

address = "United States",

edition = "1",

note = "15th International Symposium on Solid Oxide Fuel Cells, SOFC, 2017, SOFC XV ; Conference date: 23-07-2017 Through 28-07-2017",

url = "http://www.electrochem.org/sofc-xv",

}

Arifin, N, Button, T & Steinberger-Wilckens, R 2017, Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs. in SC Singhal & T Kawada (eds), Proceedings of SOFC XV. 1 edn, vol. 78, ECS Transactions, no. 1, vol. 78, Electrochemical Society Inc., Pennington, pp. 1417-1426, 15th International Symposium on Solid Oxide Fuel Cells, SOFC, 2017, Hollywood, United States, 23/07/17.

Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs. / Arifin, Nor; Button, Timothy; Steinberger-Wilckens, Robert.
Proceedings of SOFC XV. ed. / Subhash C. Singhal; T. Kawada. Vol. 78 1. ed. Pennington: Electrochemical Society Inc., 2017. p. 1417-1426 (ECS Transactions; Vol. 78, No. 1).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

TY - GEN

T1 - Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs

AU - Arifin, Nor

AU - Button, Timothy

AU - Steinberger-Wilckens, Robert

PY - 2017/7/23

Y1 - 2017/7/23

N2 - Nickel-Yttria stabilized zirconia (Ni/8YSZ) and Nickel Ceria doped-Scandia stabilised zirconia (Ni/10ScCeSZ) anode supported cells were successfully fabricated using a reverse aqueous tape casting method. The performance of the full cells were tested using both hydrogen and dry biogas at the anode side and ambient air at the cathode side in the temperature range 750°C to 800°C. In hydrogen, Ni/10ScCeSZ showed better performance at 800°C compared to the Ni/8YSZ cell. Switching the fuel from hydrogen to dry biogas, the performance of the Ni/8YSZ cell reduced significantly from 0.31 W/cm2 to 0.06 W/cm2. With Ni/10ScCeSZ cells, the cell performance in biogas was 4 times higher than the corresponding Ni8YSZ cells. The maximum power density decreased only from 0.36 W/cm2 to 0.22 W/cm2 in Ni/10ScCeSZ cell tested when switched from hydrogen to biogas. The results of this work indicate the possibility of using biogas or other carbonaceous fuel in SOFCs without the addition of water (steam).

AB - Nickel-Yttria stabilized zirconia (Ni/8YSZ) and Nickel Ceria doped-Scandia stabilised zirconia (Ni/10ScCeSZ) anode supported cells were successfully fabricated using a reverse aqueous tape casting method. The performance of the full cells were tested using both hydrogen and dry biogas at the anode side and ambient air at the cathode side in the temperature range 750°C to 800°C. In hydrogen, Ni/10ScCeSZ showed better performance at 800°C compared to the Ni/8YSZ cell. Switching the fuel from hydrogen to dry biogas, the performance of the Ni/8YSZ cell reduced significantly from 0.31 W/cm2 to 0.06 W/cm2. With Ni/10ScCeSZ cells, the cell performance in biogas was 4 times higher than the corresponding Ni8YSZ cells. The maximum power density decreased only from 0.36 W/cm2 to 0.22 W/cm2 in Ni/10ScCeSZ cell tested when switched from hydrogen to biogas. The results of this work indicate the possibility of using biogas or other carbonaceous fuel in SOFCs without the addition of water (steam).

KW - SOFC

KW - tape casting

KW - anode supported SOFC

KW - planar SOFC

KW - aqueous tape casting

KW - Carbon deposition

UR - http://toc.proceedings.com/35371webtoc.pdf

M3 - Conference contribution

SN - 978-1-60768-815-0

VL - 78

T3 - ECS Transactions

SP - 1417

EP - 1426

BT - Proceedings of SOFC XV

A2 - Singhal, Subhash C.

A2 - Kawada, T.

PB - Electrochemical Society Inc.

CY - Pennington

T2 - 15th International Symposium on Solid Oxide Fuel Cells, SOFC, 2017

Y2 - 23 July 2017 through 28 July 2017

ER -

Carbon-Tolerant Ni/ScCeSZ Via Aqueous Tape Casting for IT- SOFCs

Abstract

Publication series

Conference

Keywords

ASJC Scopus subject areas

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