A mechanism for non-stoichiometry in the lithium amide/lithium imide hydrogen storage reaction
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Colleges, School and Institutes
We demonstrate, through structural refinement from synchrotron X-ray diffraction data, that the mechanism of the transformation between lithium amide and lithium imide during hydrogen cycling in the important Li-N-H hydrogen storage system is a bulk reversible reaction that occurs in a non-stoichiometric manner within the cubic anti-fluorite-like Li-N-H structure.
|Number of pages||8|
|Journal||Journal of the American Chemical Society|
|Publication status||Published - 1 Feb 2007|