Superelongation of Liquid Metal

Xiangpeng Li, Lu Cao, Bing Xiao, Fangxia Li, Junhui Yang, Jie Hu, Tim Cole, Yuxin Zhang, Mingkui Zhang, Jiahao Zheng, Shiwu Zhang, Weihua Li, Lining Sun, Xiaoqian Chen, Shiyang Tang

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The ability to control interfacial tension electrochemically is uniquely available for liquid metals (LMs), in particular gallium-based LM alloys. This imparts them with excellent locomotion and deformation capabilities and enables diverse applications. However, electrochemical oxidation of LM is a highly dynamic process, which often induces Marangoni instabilities that make it almost impossible to elongate LM and manipulate its morphology directly and precisely on a 2D plane without the assistance of other patterning methods. To overcome these limitations, this study investigates the use of an LM–iron (Fe) particle mixture that is capable of suppressing instabilities during the electrochemical oxidation process, thereby allowing for superelongation of the LM core of the mixture to form a thin wire that is tens of times of its original length. More importantly, the elongated LM core can be manipulated freely on a 2D plane to form complex patterns. Eliminating Marangoni instabilities also allows for the effective spreading and filling of the LM–Fe mixture into molds with complex structures and small features. Harnessing these excellent abilities, a channel-less patterning method for fabricating elastomeric wearable sensors is demonstrated to detect motions. This study shows the potential for developing functional and flexible structures of LM with superior performance.
Original languageEnglish
Article number2105289
JournalAdvanced Science
Issue number11
Early online date7 Feb 2022
Publication statusE-pub ahead of print - 7 Feb 2022


  • Galinstan
  • Marangoni instabilities
  • elongation
  • liquid metal
  • wearable sensors


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