Resonance-Amplified Terahertz Near-Field Spectroscopy of a Single Nanowire

Sarah Norman*, Greg Chu, Kun Peng, James Seddon, Lucy L. Hale, Hark Hoe Tan, Chennupati Jagadish, Ralf Mouthaan, Jack Alexander-Webber, Hannah J. Joyce, Michael B. Johnston, Oleg Mitrofanov*, Thomas Siday

*Corresponding author for this work

Research output: Contribution to journalLetterpeer-review

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Abstract

Nanoscale material systems are central to next-generation optoelectronic and quantum technologies, yet their development remains hindered by limited characterization tools, particularly at terahertz (THz) frequencies. Far-field THz spectroscopy techniques lack the sensitivity for investigating individual nanoscale systems, whereas in near-field THz nanoscopy, surface states, disorder, and sample-tip interactions often mask the response of the entire nanoscale system. Here, we present a THz resonance-amplified near-field spectroscopy technique that can detect subtle conductivity changes in isolated nanoscale systems─such as a single InAs nanowire─under ultrafast photoexcitation. By exploiting the spatial localization and resonant field enhancement in the gap of a bowtie antenna, our approach enables precise measurements of the nanostructures through shifts in the antenna resonant frequency, offering a direct means of extracting the system response, and unlocking investigations of ultrafast charge-carrier dynamics in isolated nanoscale and microscale systems.

Original languageEnglish
Pages (from-to)15716-15723
Number of pages8
JournalNano Letters
Volume24
Issue number49
Early online date26 Nov 2024
DOIs
Publication statusPublished - 11 Dec 2024

Bibliographical note

Copyright:
© 2024 The Authors. Published by American Chemical Society.

Keywords

  • Nanowires
  • Near-field microscopy
  • Terahertz spectroscopy
  • Ultrafast dynamics

ASJC Scopus subject areas

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Condensed Matter Physics
  • Mechanical Engineering

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